Highly selective photocatalytic CO<sub>2</sub> reduction <i>via</i> a lead-free perovskite/MOF catalyst

نویسندگان

چکیده

A lead-free perovskite/MOF catalyst shows a high CO selectivity of 99.5% for photocatalytic 2 reduction, stemming from efficient charge separation, formation *COOH intermediates, and prompt desorptionof the catalyst.

برای دانلود رایگان متن کامل این مقاله و بیش از 32 میلیون مقاله دیگر ابتدا ثبت نام کنید

اگر عضو سایت هستید لطفا وارد حساب کاربری خود شوید

منابع مشابه

Highly cis-selective and lead-free hydrogenation of 2-hexyne by a supported Pd catalyst with an ionic-liquid layer.

A simple Pd/SiO2 catalyst which was modified with the ionic liquid [BMPL][DCA] gave an excellent yield of 88% towards cis-2-hexene in the stereoselective hydrogenation of 2-hexyne. The catalyst outperforms, even at full conversion, the commonly used lead-poisoned, toxic Lindlar catalyst and supported colloidal-based Pd as well.

متن کامل

Photocatalytic CO2 reduction using a Mn complex as a catalyst.

A photocatalytic system with a Mn(I) complex as a catalyst and a Ru(II) complex as a photosensitizer efficiently reduced CO2 to formic acid.

متن کامل

A Highly Selective Vanadium Catalyst for Benzylic C-H Oxidation.

Vanadium complexes have been used extensively to catalyze olefin and alcohol oxidation. However, their application in C-H oxidation has not been well-studied. We report herein that commercially available Cp(2)VCl(2) catalyzes benzylic C-H oxidation selectively and effectively, giving no aromatic oxidation products.

متن کامل

A dual site catalyst for mild, selective nitrile reduction.

We report a novel ruthenium bis(pyrazolyl)borate scaffold that enables cooperative reduction reactivity in which boron and ruthenium centers work in concert to effect selective nitrile reduction. The pre-catalyst compound [κ(3)-(1-pz)2HB(N = CHCH3)]Ru(cymene)(+) TfO(-) (pz = pyrazolyl) was synthesized using readily-available materials through a straightforward route, thus making it an appealing...

متن کامل

ذخیره در منابع من


  با ذخیره ی این منبع در منابع من، دسترسی به آن را برای استفاده های بعدی آسان تر کنید

ژورنال

عنوان ژورنال: Journal of materials chemistry. A, Materials for energy and sustainability

سال: 2023

ISSN: ['2050-7488', '2050-7496']

DOI: https://doi.org/10.1039/d2ta09777j